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Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent

Authorized Users Only
2018
Authors
Sajjadi, Seyed-Ali
Mohammadzadeh, Alireza
Hai, Nguyen Tran
Anastopoulos, Ioannis
Dotto, Guilherme L.
Lopičić, Zorica
Sivamani, Selvaraju
Rahmani-Sani, Abolfazl
Ivanets, Andrei
Hosseini-Bandegharaei, Ahmad
Article (Published version)
Metadata
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Abstract
Ammonium nitrate (NH4NO3) with explosive characteristics at high temperatures was used as a novel activating reagent to prepare a surface-engineered activated carbon derived from pistachio wood wastes (PWAC). PWAC was characterized and compared with commercial activated carbon (CAC) by textural and morphological properties, surface chemistry, crystal structure, and surface elemental composition. The results indicated that the optimal conditions of PWAC preparation to obtain the highest mercury adsorption capacity were pyrolysis temperature (800 degrees C), pyrolysis time (2 h), and impregnation ratio (5%). PWAC was of highly regular-shaped and well-developed pores and possessed a large surface area (1448 m(2)/g) and high total pore volume (0.901 cm(3)/g). The batch experiments indicated that the adsorption process of Hg(II) was strongly dependent on the solution pH and reached fast equilibrium at approximately 30 min. PWAC (202 mg/g) exhibited a significantly higher maximum adsorption ...capacity than commercial activated carbon (66.5 mg/g). Adsorbent-adsorbate dispersion interaction plays a major role in the adsorption mechanism, compared to the minor role played by pore filling and reduction mechanism. Overall, ammonium nitrate can be considered a newer activating reagent to prepare promising and low-cost PWAC for effectively Hg(II) removal from water media.

Keywords:
Mercury / Chemical activation / Ammonium nitrate / Agricultural waste / Adsorption / Activated carbon
Source:
Journal of Environmental Management, 2018, 223, 1001-1009
Publisher:
  • Academic Press Ltd- Elsevier Science Ltd, London
Funding / projects:
  • Central Research Council of Gonabad University of Medical Sciences

DOI: 10.1016/j.jenvman.2018.06.077

ISSN: 0301-4797

PubMed: 30096741

WoS: 000442057500102

Scopus: 2-s2.0-85049996044
[ Google Scholar ]
99
14
URI
https://ritnms.itnms.ac.rs/handle/123456789/467
Collections
  • Radovi istraživača / Researchers’ publications
Institution/Community
Institut za tehnologiju nuklearnih i drugih mineralnih sirovina
TY  - JOUR
AU  - Sajjadi, Seyed-Ali
AU  - Mohammadzadeh, Alireza
AU  - Hai, Nguyen Tran
AU  - Anastopoulos, Ioannis
AU  - Dotto, Guilherme L.
AU  - Lopičić, Zorica
AU  - Sivamani, Selvaraju
AU  - Rahmani-Sani, Abolfazl
AU  - Ivanets, Andrei
AU  - Hosseini-Bandegharaei, Ahmad
PY  - 2018
UR  - https://ritnms.itnms.ac.rs/handle/123456789/467
AB  - Ammonium nitrate (NH4NO3) with explosive characteristics at high temperatures was used as a novel activating reagent to prepare a surface-engineered activated carbon derived from pistachio wood wastes (PWAC). PWAC was characterized and compared with commercial activated carbon (CAC) by textural and morphological properties, surface chemistry, crystal structure, and surface elemental composition. The results indicated that the optimal conditions of PWAC preparation to obtain the highest mercury adsorption capacity were pyrolysis temperature (800 degrees C), pyrolysis time (2 h), and impregnation ratio (5%). PWAC was of highly regular-shaped and well-developed pores and possessed a large surface area (1448 m(2)/g) and high total pore volume (0.901 cm(3)/g). The batch experiments indicated that the adsorption process of Hg(II) was strongly dependent on the solution pH and reached fast equilibrium at approximately 30 min. PWAC (202 mg/g) exhibited a significantly higher maximum adsorption capacity than commercial activated carbon (66.5 mg/g). Adsorbent-adsorbate dispersion interaction plays a major role in the adsorption mechanism, compared to the minor role played by pore filling and reduction mechanism. Overall, ammonium nitrate can be considered a newer activating reagent to prepare promising and low-cost PWAC for effectively Hg(II) removal from water media.
PB  - Academic Press Ltd- Elsevier Science Ltd, London
T2  - Journal of Environmental Management
T1  - Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent
EP  - 1009
SP  - 1001
VL  - 223
DO  - 10.1016/j.jenvman.2018.06.077
UR  - conv_831
ER  - 
@article{
author = "Sajjadi, Seyed-Ali and Mohammadzadeh, Alireza and Hai, Nguyen Tran and Anastopoulos, Ioannis and Dotto, Guilherme L. and Lopičić, Zorica and Sivamani, Selvaraju and Rahmani-Sani, Abolfazl and Ivanets, Andrei and Hosseini-Bandegharaei, Ahmad",
year = "2018",
abstract = "Ammonium nitrate (NH4NO3) with explosive characteristics at high temperatures was used as a novel activating reagent to prepare a surface-engineered activated carbon derived from pistachio wood wastes (PWAC). PWAC was characterized and compared with commercial activated carbon (CAC) by textural and morphological properties, surface chemistry, crystal structure, and surface elemental composition. The results indicated that the optimal conditions of PWAC preparation to obtain the highest mercury adsorption capacity were pyrolysis temperature (800 degrees C), pyrolysis time (2 h), and impregnation ratio (5%). PWAC was of highly regular-shaped and well-developed pores and possessed a large surface area (1448 m(2)/g) and high total pore volume (0.901 cm(3)/g). The batch experiments indicated that the adsorption process of Hg(II) was strongly dependent on the solution pH and reached fast equilibrium at approximately 30 min. PWAC (202 mg/g) exhibited a significantly higher maximum adsorption capacity than commercial activated carbon (66.5 mg/g). Adsorbent-adsorbate dispersion interaction plays a major role in the adsorption mechanism, compared to the minor role played by pore filling and reduction mechanism. Overall, ammonium nitrate can be considered a newer activating reagent to prepare promising and low-cost PWAC for effectively Hg(II) removal from water media.",
publisher = "Academic Press Ltd- Elsevier Science Ltd, London",
journal = "Journal of Environmental Management",
title = "Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent",
pages = "1009-1001",
volume = "223",
doi = "10.1016/j.jenvman.2018.06.077",
url = "conv_831"
}
Sajjadi, S., Mohammadzadeh, A., Hai, N. T., Anastopoulos, I., Dotto, G. L., Lopičić, Z., Sivamani, S., Rahmani-Sani, A., Ivanets, A.,& Hosseini-Bandegharaei, A.. (2018). Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent. in Journal of Environmental Management
Academic Press Ltd- Elsevier Science Ltd, London., 223, 1001-1009.
https://doi.org/10.1016/j.jenvman.2018.06.077
conv_831
Sajjadi S, Mohammadzadeh A, Hai NT, Anastopoulos I, Dotto GL, Lopičić Z, Sivamani S, Rahmani-Sani A, Ivanets A, Hosseini-Bandegharaei A. Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent. in Journal of Environmental Management. 2018;223:1001-1009.
doi:10.1016/j.jenvman.2018.06.077
conv_831 .
Sajjadi, Seyed-Ali, Mohammadzadeh, Alireza, Hai, Nguyen Tran, Anastopoulos, Ioannis, Dotto, Guilherme L., Lopičić, Zorica, Sivamani, Selvaraju, Rahmani-Sani, Abolfazl, Ivanets, Andrei, Hosseini-Bandegharaei, Ahmad, "Efficient mercury removal from wastewater by pistachio wood wastes-derived activated carbon prepared by chemical activation using a novel activating agent" in Journal of Environmental Management, 223 (2018):1001-1009,
https://doi.org/10.1016/j.jenvman.2018.06.077 .,
conv_831 .

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