Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia
Само за регистроване кориснике
2020
Аутори
Ranđelović, DraganaMutić, Jelena
Marjanović, Prvoslav
Đorđević, Tamara
Kasanin-Grubin, Milica
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobi...lity can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill.
Кључне речи:
Soil / Risk assessment / Metal(oid)s / Flotation tailings spillИзвор:
Environmental science and pollution research, 2020, 27, 6, 6253-6268Издавач:
- Springer Heidelberg, Heidelberg
Финансирање / пројекти:
- Магматизам и геодинамика Балканског полуострва од мезозоика до данас: значај за образовање металичних и неметаличних рудних лежишта (RS-MESTD-Basic Research (BR or ON)-176016)
- Примена унапређених оксидационих процеса и наноструктурисаних оксидних материјала за уклањање загађивача из животне средине, развој и оптимизација инструменталних техника за праћење ефикасности (RS-MESTD-Basic Research (BR or ON)-172030)
- Геохемијска испитивања седиментних стена - фосилна горива и загађивачи животне средине (RS-MESTD-Basic Research (BR or ON)-176006)
DOI: 10.1007/s11356-019-07348-4
ISSN: 0944-1344
PubMed: 31863383
WoS: 000503669600003
Scopus: 2-s2.0-85077063885
Институција/група
Institut za tehnologiju nuklearnih i drugih mineralnih sirovinaTY - JOUR AU - Ranđelović, Dragana AU - Mutić, Jelena AU - Marjanović, Prvoslav AU - Đorđević, Tamara AU - Kasanin-Grubin, Milica PY - 2020 UR - https://ritnms.itnms.ac.rs/handle/123456789/533 AB - Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobility can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill. PB - Springer Heidelberg, Heidelberg T2 - Environmental science and pollution research T1 - Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia EP - 6268 IS - 6 SP - 6253 VL - 27 DO - 10.1007/s11356-019-07348-4 UR - conv_870 ER -
@article{ author = "Ranđelović, Dragana and Mutić, Jelena and Marjanović, Prvoslav and Đorđević, Tamara and Kasanin-Grubin, Milica", year = "2020", abstract = "Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobility can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill.", publisher = "Springer Heidelberg, Heidelberg", journal = "Environmental science and pollution research", title = "Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia", pages = "6268-6253", number = "6", volume = "27", doi = "10.1007/s11356-019-07348-4", url = "conv_870" }
Ranđelović, D., Mutić, J., Marjanović, P., Đorđević, T.,& Kasanin-Grubin, M.. (2020). Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia. in Environmental science and pollution research Springer Heidelberg, Heidelberg., 27(6), 6253-6268. https://doi.org/10.1007/s11356-019-07348-4 conv_870
Ranđelović D, Mutić J, Marjanović P, Đorđević T, Kasanin-Grubin M. Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia. in Environmental science and pollution research. 2020;27(6):6253-6268. doi:10.1007/s11356-019-07348-4 conv_870 .
Ranđelović, Dragana, Mutić, Jelena, Marjanović, Prvoslav, Đorđević, Tamara, Kasanin-Grubin, Milica, "Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia" in Environmental science and pollution research, 27, no. 6 (2020):6253-6268, https://doi.org/10.1007/s11356-019-07348-4 ., conv_870 .